I have never seen bit rot first hand. Only once have I experienced a disc not playing a certain track due to a scratch (it was track 10 on Street Fighter II Alph Lyla with Yuji Toriyama). I have had many problems with burned media, but that's to be expected.
I would suspect that if anyone can build the largest soundtrack collection, it would be the youtuber The Last Gamer. He seems to have the space and the resources to make it happen. For logistical reasons, until some maniac like The Last Gamer tries to set another record, the largest collection is probably somewhere in Japan.
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